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Jürgen P. Rabe

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Jürgen P. Rabe is a German physicist and nanoscientist.

Life

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Jürgen P. Rabe studied physics and mathematics at RWTH Aachen where in 1981 he obtained his diploma in physics, based on a thesis on semiconductor optics with Peter Grosse. 1984 he obtained his doctoral degree from the Department of Physics at the Technische Universität München, based on a biophysical thesis on model membranes, promoted by Erich Sackmann.

As a visiting scientist at the IBM Almaden Research Center in San José (1984–1986) he initiated the use of scanning tunneling microscopy for molecular monolayers, which he continued in Gerhard Wegner’s department at the Max Planck Institute for Polymer Research.

In 1992 he obtained his habilitation[1] on this topic and became a professor for physical chemistry at Johannes Gutenberg-Universität in Mainz. Since 1994 Rabe is full professor for experimental physics with an emphasis on macromolecular and supramolecular systems at the Department of Physics at the Humboldt-Universität zu Berlin. Rabe is an elected scientific member of the Max Planck Society and external member of the Max Planck Institute of Colloids and Interfaces in Potsdam-Golm as well as founding director of the Integrative Research Institute for the Sciences IRIS Adlershof of Humboldt-Universität. He was visiting professor at the Materials Department of ETH Zürich and for the Department of Chemistry at Princeton University.

Jürgen P. Rabe is the brother of Klaus F. Rabe and cousin of Sophia Rabe-Hesketh and the economist Birgitta Rabe.

Research

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Rabe became internationally known for his seminal scanning tunneling microscopy research on the structure, dynamics, and electronic properties of self-assembled molecular systems at solid-liquid interfaces.[2][3][4][5][6][7][8] He developed concepts for a workbench to manipulate individual macromolecules and supramolecular systems, employing scanning probe microscopies, light, and molecularly modified graphite surfaces,[9] which has been used to correlate structure and dynamics of molecular systems with mechanical, electronic, optical, and (bio)chemical properties from molecular to macromolecular lengths and time scales.[10][11] It also led to the development of prototypical quasi 1- and 2- dimensional organic-inorganic hybrid systems, based on opto-electronically active molecular or graphene-based nanopores.[12][13][14][15][16][17] In collaborative and interdisciplinary projects Rabe contributed to the development of advanced functional materials, including dendronized[18][19] and conjugated polymers,[20] multivalent biopolymer complexes,[21][22] ultrathin films of conjugated molecules,[23][24][25] supramolecular polymers[26] and helical nanofilaments,[27] nanographenes,[5][7] and 2D materials[28][29][30] as well as mixed 2D/3D heterostructures.[31]

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References

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  1. ^ http://d-nb.info/943087414 Raster-Tunnelmikroskopie organischer Monoschichten : Struktur, Dynamik und elektronische Eigenschaften auf molekularer Skala / Jürgen P. Rabe
  2. ^ Rabe, Jürgen P.; Buchholz, Stefan (1991-07-12). "Commensurability and Mobility in Two-Dimensional Molecular Patterns on Graphite". Science. 253 (5018): 424–427. Bibcode:1991Sci...253..424R. doi:10.1126/science.253.5018.424. ISSN 0036-8075. PMID 17746397. S2CID 42385720.
  3. ^ Rabe, Jürgen P.; Buchholz, Stefan (1991). "Direct observation of molecular structure and dynamics at the interface between a solid wall and an organic solution by scanning tunneling microscopy". Physical Review Letters. 66 (16): 2096–2099. Bibcode:1991PhRvL..66.2096R. doi:10.1103/physrevlett.66.2096. PMID 10043390.
  4. ^ Hentschke, Reinhard; Schürmann, Britta L.; Rabe, Jürgen P. (1992-04-15). "Molecular dynamics simulations of ordered alkane chains physisorbed on graphite". The Journal of Chemical Physics. 96 (8): 6213–6221. Bibcode:1992JChPh..96.6213H. doi:10.1063/1.462612. ISSN 0021-9606.
  5. ^ a b Stabel, Andreas; Herwig, Peter; Müllen, Klaus; Rabe, Jürgen P. (1995-08-18). "Diodelike Current–Voltage Curves for a Single Molecule–Tunneling Spectroscopy with Submolecular Resolution of an Alkylated, peri-Condensed Hexabenzocoronene". Angewandte Chemie International Edition in English. 34 (15): 1609–1611. doi:10.1002/anie.199516091. ISSN 1521-3773.
  6. ^ Jäckel, Frank; Watson, Mark D.; Müllen, Klaus; Rabe, Jürgen P. (2004-5-6). "Prototypical single molecule chemical field effect transistor with nanometer-sized gates". Physical Review Letters. 92 (18). doi:10.1103/PhysRevLett.92.188303. Featured by Auweraer, M. Van der; Schryver, F. C. De. "Organic electronics: Supra solutions". Nature Materials. 3 (8): 507–508. doi:10.1038/nmat1182.M.
  7. ^ a b Müllen, Klaus; Rabe, Jürgen P. (2008-04-01). "Nanographenes as Active Components of Single-Molecule Electronics and How a Scanning Tunneling Microscope Puts Them To Work". Accounts of Chemical Research. 41 (4): 511–520. doi:10.1021/ar7001446. ISSN 0001-4842. PMID 18410086.
  8. ^ Cojal González, José D.; Iyoda, Masahiko; Rabe, Jürgen P. (2017-03-10). "Templated bilayer self-assembly of fully conjugated π-expanded macrocyclic oligothiophenes complexed with fullerenes". Nature Communications. 8: ncomms14717. Bibcode:2017NatCo...814717C. doi:10.1038/ncomms14717. PMC 5353715. PMID 28281557.
  9. ^ Rabe, Jürgen P. (2008). "Molecular workbench for imaging and manipulation of single macromolecules and their complexes with the scanning force microscope". In Samorì, Paolo (ed.). STM and AFM Studies on (Bio)molecular Systems: Unravelling the Nanoworld. Topics in Current Chemistry. Vol. 285. Springer, Berlin, Heidelberg. pp. 77–102. doi:10.1007/128_2008_4. ISBN 978-3-540-78395-4. PMID 23636676.
  10. ^ Barner, Jörg; Mallwitz, Frank; Shu, Lijin; Schlüter, A. Dieter; Rabe, Jürgen P. (2003-04-29). "Covalent Connection of Two Individual Polymer Chains on a Surface: An Elementary Step towards Molecular Nanoconstructions". Angewandte Chemie International Edition. 42 (17): 1932–1935. doi:10.1002/anie.200250059. ISSN 1521-3773. PMID 12730972.
  11. ^ Lee, Chien-Li; Liebig, Tobias; Hecht, Stefan; Bléger, David; Rabe, Jürgen P. (2014-12-23). "Light-Induced Contraction and Extension of Single Macromolecules on a Modified Graphite Surface". ACS Nano. 8 (12): 11987–11993. ISSN 1936-0851. doi:10.1021/nn505325w. Featured in Kundu, Pintu K.; Klajn, Rafal (2014-12-23). "Watching Single Molecules Move in Response to Light". ACS Nano. 8 (12): 11913–11916. ISSN 1936-0851. doi:10.1021/nn506656r.
  12. ^ Eisele, Dörthe M.; Knoester, Jasper; Kirstein, Stefan; Rabe, Jürgen P.; Vanden Bout, David A. (2009). "Uniform exciton fluorescence from individual molecular nanotubes immobilized on solid substrates" (PDF). Nature Nanotechnology. 4 (10): 658–663. Bibcode:2009NatNa...4..658E. doi:10.1038/nnano.2009.227. hdl:11370/7815fb76-b75e-4ea5-800a-f6e6bcc3d029. PMID 19809457.
  13. ^ Qiao, Yan; Polzer, Frank; Kirmse, Holm; Steeg, Egon; Kühn, Sergei; Friede, Sebastian; Kirstein, Stefan; Rabe, Jürgen P. (2015-02-24). "Nanotubular J-Aggregates and Quantum Dots Coupled for Efficient Resonance Excitation Energy Transfer". ACS Nano. 9 (2): 1552–1560. doi:10.1021/nn506095g. ISSN 1936-0851. PMID 25555126.
  14. ^ Steeg, Egon; Kirmse, Holm; Rabe, Jürgen P.; Kirstein, Stefan (2015-02-24). "Silver iodide nanowires grown within tubular J-aggregates". Journal of Colloid and Interface Science. 530: 424–432. doi:10.1016/j.jcis.2018.06.099. ISSN 0021-9797. PMID 29990778. S2CID 51618319.
  15. ^ Severin, Nikolai; Lange, Philipp; Sokolov, Igor M.; Rabe, Jürgen P. (2012-02-08). "Reversible Dewetting of a Molecularly Thin Fluid Water Film in a Soft Graphene–Mica Slit Pore". Nano Letters. 12 (2): 774–779. Bibcode:2012NanoL..12..774S. doi:10.1021/nl2037358. ISSN 1530-6984. PMID 22216882.
  16. ^ Lin, Hu; Schilo, Andre; Kamoka, A. Rauf; Severin, Nikolai; Sokolov, Igor M.; Rabe, Jürgen P. (2017). "Insight into the wetting of a graphene-mica slit pore with a monolayer of water". Physical Review B. 95 (19): 195414. Bibcode:2017PhRvB..95s5414L. doi:10.1103/physrevb.95.195414.
  17. ^ Lin, Wan-Ing; Gholami, M. Fardin; Beyer, Paul; Severin, Nikolai; Shao, Feng; Zenobi, Renato; Rabe, Jürgen P. (2017-01-05). "Strongly enhanced Raman scattering of Cu-phthalocyanine sandwiched between graphene and Au(111)". Chem. Commun. 53 (4): 724–727. doi:10.1039/c6cc08672a. ISSN 1364-548X. PMID 27990530.
  18. ^ Schlüter, A. Dieter; Rabe, Jürgen P. (2000-03-03). "Dendronized Polymers: Synthesis, Characterization, Assembly at Interfaces, and Manipulation". Angewandte Chemie International Edition. 39 (5): 864–883. doi:10.1002/(sici)1521-3773(20000303)39:5<864::aid-anie864>3.0.co;2-e. ISSN 1521-3773. PMID 10760880.
  19. ^ Gössl, Illdiko; Shu, Lijin; Schlüter, A. Dieter; Rabe, Jürgen P. (2002-06-01). "Molecular Structure of Single DNA Complexes with Positively Charged Dendronized Polymers". Journal of the American Chemical Society. 124 (24): 6860–6865. doi:10.1021/ja017828l. ISSN 0002-7863. PMID 12059206.
  20. ^ Zen, Achmad; Pflaum, Jens; Hirschmann, S.; Zhuang, Wei; Jaiser, Frank; Asawapirom, Udom; Rabe, Jürgen P.; Scherf, Ullrich; Neher, Dieter (2004-08-01). "Effect of Molecular Weight and Annealing of Poly(3-hexylthiophene)s on the Performance of Organic Field-Effect Transistors". Advanced Functional Materials. 14 (8): 757–764. doi:10.1002/adfm.200400017. ISSN 1616-3028. S2CID 98257664.
  21. ^ Reiter-Scherer, Valentin; Cuellar-Camacho, Jose Luis; Bhatia, Sumati; Haag, Rainer; Herrmann, Andreas; Lauster, Daniel; Rabe, Jürgen P. (2019-02-08). "Force Spectroscopy Shows Dynamic Binding of Influenza Hemagglutinin and Neuraminidase to Sialic Acid". Biophysical Journal. 116 (8): 1037–1048. Bibcode:2019BpJ...116.1037R. doi:10.1016/j.bpj.2019.01.041. ISSN 0006-3495. PMC 6428919. PMID 30799074.
  22. ^ Cuellar-Camacho, Jose Luis; Bhatia, Sumati; Reiter-Scherer, Valentin; Lauster, Daniel; Liese, Susanne; Rabe, Jürgen P.; Herrmann, Andreas; Haag, Rainer (2020-06-14). "Quantification of Multivalent Interactions between Sialic Acid and Influenza A Virus Spike Proteins by Single-Molecule Force Spectroscopy". Journal of the American Chemical Society. 142 (28): 12181–12192. doi:10.1021/jacs.0c02852. PMID 32538085. S2CID 219702891.
  23. ^ Koch, Norbert; Duhm, Steffen; Rabe, Jürgen P.; Vollmer, Antje; Johnson, Robert L. (2005). "Optimized Hole Injection with Strong Electron Acceptors at Organic-Metal Interfaces" (PDF). Physical Review Letters. 95 (23): 237601. Bibcode:2005PhRvL..95w7601K. doi:10.1103/physrevlett.95.237601. PMID 16384346.
  24. ^ Koch, Norbert; Vollmer, Antje; Salzmann, Ingo; Nickel, Bert; Weiss, Helmut; Rabe, Jürgen P. (2006). "Evidence for Temperature-Dependent Electron Band Dispersion in Pentacene". Physical Review Letters. 96 (15): 156803. Bibcode:2006PhRvL..96o6803K. doi:10.1103/physrevlett.96.156803. PMID 16712184.
  25. ^ Duhm, Steffen; Heimel, Georg; Salzmann, Ingo; Glowatzki, Hendrik; Johnson, Robert L.; Vollmer, Antje; Rabe, Jürgen P.; Koch, Norbert (2008). "Orientation-dependent ionization energies and interface dipoles in ordered molecular assemblies" (PDF). Nature Materials. 7 (4): 326–332. Bibcode:2008NatMa...7..326D. doi:10.1038/nmat2119. PMID 18264103. S2CID 19548874.
  26. ^ Cacialli, Franco; Wilson, Joanne S.; Michels, Jasper J.; Daniel, Clement; Silva, Carlos; Friend, Richard H.; Severin, Nikolai; Samorì, Paolo; Rabe, Jürgen P.; O'Connell, Michael J.; Taylor, Peter N.; Anderson, Harry L. (2002). "Cyclodextrin-threaded conjugated polyrotaxanes as insulated molecular wires with reduced interstrand interactions". Nature Materials. 1 (3): 160–164. Bibcode:2002NatMa...1..160C. doi:10.1038/nmat750. PMID 12618803. S2CID 15401769.
  27. ^ Hough, Loren E.; Jung, Hee-Tae; Krüerke, Daniel; Heberling, M. S.; Nakata, Michi; Jones, Christopher D.; Chen, Dong; Link, Darren R.; Zasadzinski, Joseph; Heppke, Gerd; Rabe, Jürgen P.; Stocker, Wolfgang; Körblova, Eva; Walba, David M.; Glaser, Matthew A.; Clark, Noel A. (2009-07-24). "Helical Nanofilament Phases". Science. 325 (5939): 456–460. Bibcode:2009Sci...325..456H. doi:10.1126/science.1170027. ISSN 0036-8075. PMID 19628864. S2CID 26379217.
  28. ^ Breusing, Markus; Kuehn, Sergei; Winzer, Torben; Malić, Ermin; Milde, Frank; Severin, Nikolai; Rabe, Jürgen P.; Ropers, Claus; Knorr, Andreas; Elsaesser, Thomas (2011). "Ultrafast nonequilibrium carrier dynamics in a single graphene layer". Physical Review B. 83 (15): 153410. Bibcode:2011PhRvB..83o3410B. doi:10.1103/physrevb.83.153410. S2CID 54840899.
  29. ^ Gholami, M. Fardin; Severin, Nikolai; Rabe, Jürgen P. (2016). "Folding of graphene and other two-dimensional materials". In Friedman, Michael; Schäffner, Wolfgang (eds.). On Folding: Towards a New Field of Interdisciplinary Research. transcript Verlag. pp. 211–237. ISBN 9783837634044. OCLC 953602819.
  30. ^ Algara-Siller, Gerardo; Severin, Nikolai; Chong, Samantha Y.; Björkman, Torbjörn; Palgrave, Robert G.; Laybourn, Andrea; Antonietti, Markus; Khimyak, Yaroslav Z.; Krasheninnikov, Arkady V.; Rabe, Jürgen P.; Kaiser, Ute; Cooper, Andrew I.; Thomas, Arne; Bojdys, Michael J. (2014-07-14). "Triazine-Based Graphitic Carbon Nitride: a Two-Dimensional Semiconductor". Angewandte Chemie International Edition. 53 (29): 7450–7455. doi:10.1002/anie.201402191. ISSN 1521-3773. PMID 24838808.
  31. ^ Schwarz, Dana; Noda, Yu; Klouda, Jan; Schwarzová-Pecková, Karolina; Tarábek, Ján; Rybáček, Jiří; Janoušek, Jiří; Simon, Frank; Opanasenko, Maksym V.; Čejka, Jiří; Acharjya, Amitava; Schmidt, Johannes; Selve, Sören; Reiter-Scherer, Valentin; Severin, Nikolai; Rabe, Jürgen P.; Ecorchard, Petra; He, Junjie; Polozij, Miroslav; Nachtigall, Petr; Bojdys, Michael J. (2017). "Twinned Growth of Metal-Free, Triazine-Based Photocatalyst Films as Mixed-Dimensional (2D/3D) van der Waals Heterostructures". Advanced Materials. 29 (40): 1703399. Bibcode:2017AdM....2903399S. doi:10.1002/adma.201703399. ISSN 1521-4095. PMID 28859235. S2CID 11009055.


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